We settle the debate on the bright-dark exciton level ordering in these materials. We show evidence for universal scaling laws relating the exciton fine structure splitting, the trion and biexciton binding energies to the band-edge exciton energy in lead-halide perovskite nanostructures, regardless of their chemical composition.
Jacky EVEN, Fonctions Optiques pour les Technologies de l’informatiON (FOTON) jacky.even insa-rennes.fr |
Claudine KATAN, Institut des Sciences Chimiques de Rennes (ISCR) claudine.katan univ-rennes1.fr |
Université de Bordeaux (France), ISCR (Rennes, France), ETH Zurich (Zurich, Switzerland)
This work was financially supported by the European Union through the Horizon 2020 Research and Innovation Programme through the Fetopen Research and Innovation Action (grant agreement no. 899141, project Polloc)
Universal scaling laws for charge-carrier interactions with quantum confinement in lead-halide perovskites, P. Tamarat, E. Prin, Y. Berezovska, A. Moskalenko, T. P. T. Nguyen, C. Xia, L. Hou, J.-B. Trebbia, M. Zacharias, L. Pedesseau, C. Katan, M. I. Bodnarchuk, M. V. Kovalenko, J. Even & B. Lounis Nat. Commun. Vol. 14, 229, 2023, hal-03125950